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Photothermal materials for efficient solar powered steam generation

Fenghua Liu, Yijian Lai, Binyuan Zhao, Robert Bradley, Weiping Wu

《化学科学与工程前沿（英文）》 2019年第13卷第4期页码 636-653 doi: 10.1007/s11705-019-1824-1

摘要： Solar powered steam generation is an emerging area in the field of energy harvest and sustainable technologies. The nano-structured photothermal materials are able to harvest energy from the full solar spectrum and convert it to heat with high efficiency. Moreover, the materials and structures for heat management as well as the mass transportation are also brought to the forefront. Several groups have reported their materials and structures as solutions for high performance devices, a few creatively coupled other physical fields with solar energy to achieve even better results. This paper provides a systematic review on the recent developments in photothermal nanomaterial discovery, material selection, structural design and mass/heat management, as well as their applications in seawater desalination and fresh water production from waste water with free solar energy. It also discusses current technical challenges and likely future developments. This article will help to stimulate novel ideas and new designs for the photothermal materials, towards efficient, low cost practical solar-driven clean water production.

关键词： solar stream generation plasmonics porous carbon photothermal materials solar energy conversion efficiency water vapor generation rate

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Ozone kinetics of dimethyl sulfide in the presence of water vapor

Haitao WANG

《环境科学与工程前沿（英文）》 2013年第7卷第6期页码 833-835 doi: 10.1007/s11783-013-0570-8

摘要： The outdoor smog chamber was used to thorough investigate the rate constants of gas-phase reaction between dimethyl sulfide (DMS) and ozone (O ) under conditions of relative humidity 55.0%–67.8% at (296±2)K for the first time. The rate constants were measured, at a total pressure of 1 atm, to be (10.4±0.2) × 10 cm ·molecule ·s at relative humidity of 67.5%±0.3% at 298K, (10.1±0.1) × 10 cm ·molecule ·s at relative humidity of 66.5%±0.5% at 296K, (7.75±0.39) × 10 cm ·molecule ·s at relative humidity of 64.8%±0.1% at 294K and (3.42±0.21) × 10 cm ·molecule ·s at relative humidity of 55.8%±0.8% at 295K. Base on these results, it is possible to see the reaction of O /DMS in the presence of water vapor as an important sink for DMS in the earth atmosphere.

关键词： rate constants ozone (O₃) dimethyl sulfide (DMS) water vapor

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Modeling of coal swelling induced by water vapor adsorption

Zhejun PAN

《化学科学与工程前沿（英文）》 2012年第6卷第1期页码 94-103 doi: 10.1007/s11705-011-1172-2

摘要： Gas adsorption-induced coal swelling is a well-know phenomenon. Coal swelling or shrinkage by adsorption or desorption of water vapor has not been well understood but has significant implications on gas drainage process for underground coal mining and for primary and enhanced coalbed methane production. Decreased matrix moisture content leads to coal shrinkage and thus the change of cleat porosity and permeability under reservoir conditions. Unlike gas adsorption in coal which usually forms a single layer of adsorbed molecules, water vapor adsorption in the coal micropores forms multilayer of adsorbed molecules. In this work, a model has been developed to describe the coal swelling strain with respect to the amount of moisture intake by the coal matrix. The model extended an energy balance approach for gas adsorption-induced coal swelling to water vapor adsorption-induced coal swelling, assuming that only the first layer of adsorbed molecules of the multilayer adsorption changes the surface energy, which thus causes coal to swell. The model is applied to describe the experimental swelling strain data measured on an Australian coal. The results show good agreement between the model and the experimental data.

关键词： multilayer adsorption vapour pressure coal shrinkage relative humidity permeability

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Thermodynamic study on dynamic water and organic vapor sorption on amorphous valnemulin hydrochloride

Jinbo OUYANG, Jingkang WANG, Yongli WANG, Qiuxiang YIN, Hongxun HAO

《化学科学与工程前沿（英文）》 2015年第9卷第1期页码 94-104 doi: 10.1007/s11705-015-1460-3

摘要： The sorption of water and organic vapors on valnemulin hydrochloride was determined by dynamic vapor sorption at 25 °C. The adsorption-desorption behavior of water vapor and a series of organic vapors was investigated to probe the structural changes in valnemulin hydrochloride before and after sorption. The isothermal adsorption equilibrium data was evaluated using Guggenheim-Anderson-deBoer (GAB) and Brunauer-Emmett-Teller (BET) models. The BET model is applicable only at low relative pressures (0.1≤RP≤0.4) while the GAB model is applicable in the whole range of RPs (0.1≤RP≤0.9). The sorption kinetics at high RPs was determined by fitting the sorption data to the Avrami equation and the sorption content time relationship could be predicted by the Avrami equation. Finally, the possible sorption mechanism of valnemulin hydrochloride was also discussed.

关键词： valnemulin hydrochloride water vapor organic vapors sorption kinetics

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Modified landfill gas generation rate model of first-order kinetics and two-stage reaction

Jiajun CHEN , Hao WANG , Na ZHANG ,

《环境科学与工程前沿（英文）》 2009年第3卷第3期页码 313-319 doi: 10.1007/s11783-009-0025-4

摘要： This investigation was carried out to establish a new domestic landfill gas (LFG) generation rate model that takes into account the impact of leachate recirculation. The first-order kinetics and two-stage reaction (FKTSR) model of the LFG generation rate includes mechanisms of the nutrient balance for biochemical reaction in two main stages. In this study, the FKTSR model was modified by the introduction of the outflow function and the organic acid conversion coefficient in order to represent the in-situ condition of nutrient loss through leachate. Laboratory experiments were carried out to simulate the impact of leachate recirculation and verify the modified FKTSR model. The model calibration was then calculated by using the experimental data. The results suggested that the new model was in line with the experimental data. The main parameters of the modified FKTSR model, including the LFG production potential (), the reaction rate constant in the first stage (), and the reaction rate constant in the second stage () of 64.746 L, 0.202 d, and 0.338 d, respectively, were comparable to the old ones of 42.069 L, 0.231 d, and 0.231 d. The new model is better able to explain the mechanisms involved in LFG generation.

关键词： landfill gas (LFG) generation rate model first-order kinetics two-stage reaction outflow function

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Studies on advanced water-cooled reactors beyond generation III for power generation

CHENG Xu

《能源前沿（英文）》 2007年第1卷第2期页码 141-149 doi: 10.1007/s11708-007-0018-6

摘要： China s ambitious nuclear power program motivates the country s nuclear community to develop advanced reactor concepts beyond generation III to ensure a long-term, stable, and sustainable development of nuclear power. The paper discusses some main criteria for the selection of future water-cooled reactors by considering the specific Chinese situation. Based on the suggested selection criteria, two new types of water-cooled reactors are recommended for future Chinese nuclear power generation. The high conversion pressurized water reactor utilizes the present PWR technology to a large extent. With a conversion ratio of about 0.95, the fuel utilization is increased about 5 times. This significantly improves the sustainability of fuel resources. The supercritical water-cooled reactor has favorable features in economics, sustainability and technology availability. It is a logical extension of the generation III PWR technology in China. The status of international R&D work is reviewed. A new supercritical water-cooled reactor (SCWR) core structure (the mixed reactor core) and a new fuel assembly design (two-rows FA) are proposed. The preliminary analysis using a coupled neutron-physics/thermal-hydraulics method is carried out. It shows good feasibility for the new design proposal.

关键词： Chinese situation selection generation water-cooled feasibility

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Facile strategy for carbon foam fabrication with lignin as sole feedstock and its applications

《化学科学与工程前沿（英文）》 2023年第17卷第8期页码 1051-1064 doi: 10.1007/s11705-022-2248-x

摘要： This research is a follow-up to our recent discovery of a facile strategy for directly converting lignin powder into carbon foam. In this work, we report that the thermal pretreatment parameters in air can remarkably influence the formation and properties of the derived carbon foam. Thermal pretreatment parameters (heating rate, temperature, and residence time) were systematically investigated and a conversion mechanism into carbon foam was proposed. During the thermal pretreatment, relatively low temperatures, low heating rates, and short residence time hindered the formation of smooth and well-connected structures in the carbon foam. The overall product yields were similar regardless of the thermal pretreatment conditions. The densities of the different carbon foams ranged 0.27–0.83 g∙cm⁻³. The carbon foams with the highest compressive strengths (> 10 MPa) were KLPC280-2-5, KLPC300-0-5, and KLPC300-2-2.5. KLPC280-2-5 exhibited a high iodine sorption value (182 mg∙g⁻¹). KLPC300-2-5 exhibited a specific capacitance of 158 F∙g⁻¹ at a current density of 0.05 A∙g⁻¹. The maximum evaporation rates in the solar vapor generation experiments were 1.05 and 1.38 kg∙m⁻²∙h⁻¹ under 100 and 150 mW∙cm⁻² irradiation, respectively. The good performances are attributed to the robust, porous, and continuous structure.

关键词： lignin carbon foam thermal pretreatment solar vapor generation

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A hybrid fuel cell for water purification and simultaneously electricity generation

《环境科学与工程前沿（英文）》 2023年第17卷第1期 doi: 10.1007/s11783-023-1611-6

摘要：

● A novel hybrid fuel cell (F-HFC) was fabricated.

关键词： Flow-through field Hybrid fuel cell Polyoxometalates Water purification Electricity generation

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垃圾填埋场气体产生及其模型研究

黄文雄,彭绪亚,阎利

《中国工程科学》 2006年第8卷第9期页码 74-79

摘要：

对填埋气的回收利用，既能减排温室气体，又能回收能源。分析了填埋气产生的原理和过程，对目前出现的填埋场产气模型进行了分类，并系统地分析了各种产气模型的计算方法、优缺点以及适用条件，为填埋气体的大规模利用提供可靠的方法。

关键词：填埋气模型产气速率产气量甲烷

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Heat transfer characteristics of high heat flux vapor chamber

Dongchuan MO, Shushen LU, Haoliang ZHENG, Chite CHIN,

《能源前沿（英文）》 2010年第4卷第2期页码 166-170 doi: 10.1007/s11708-009-0076-z

摘要： To meet the challenge of heat spreading in electronic products, highly efficient high heat flux heat transfer vapor chambers have been manufactured and their heat transfer characteristics have been studied by a fast test system. A solid copper block with the same shape as the vapor chamber is used to compare the performance of the vapor chamber. The result shows that, it will take about 5min to achieve a steady state in the fast test system. The heat transfer characteristics of the vapor chamber are more superior to those of the copper block. In this paper, total thermal resistance of the test system is used to evaluate the heat transfer characteristics of the vapor chamber, because it has already been used to consider both the spreading thermal resistance and the flatness of the vapor chamber.

关键词： high heat flux vapor chamber (VC) heat transfer characteristics fast test

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Metal-based direct hydrogen generation as unconventional high density energy

Shuo XU, Jing LIU

《能源前沿（英文）》 2019年第13卷第1期页码 27-53 doi: 10.1007/s11708-018-0603-x

摘要： Metals are unconventional hydrogen production materials which are of high energy densities. This paper comprehensively reviewed and digested the latest researches of the metal-based direct hydrogen generation and the unconventional energy utilization ways thus enabled. According to the metal activities, the reaction conditions of metals were generalized into three categories. The first ones refer to those which would violently react with water at ambient temperature. The second ones start to react with water after certain pretreatments. The third ones can only react with steam under somewhat harsh conditions. To interpret the metal-water reaction mechanisms at the molecular scale, the molecule dynamics simulation and computational quantum chemistry were introduced as representative theoretical analytical tools. Besides, the state-of-the-art of the metal-water reaction was presented with several ordinary metals as illustration examples, including the material treatment technologies and the evaluations of hydrogen evolution performances. Moreover, the energy capacities of various metals were summarized, and the application potentials of the metal-based direct hydrogen production approach were explored. Furthermore, the challenges lying behind this unconventional hydrogen generation method and energy strategy were raised, which outlined promising directions worth of further endeavors. Overall, active metals like Na and K are appropriate for rapid hydrogen production occasions. Of these metals discussed, Al, Mg and their alloys offer the most promising hydrogen generation route for clean and efficient propulsion and real-time power source. In the long run, there exists plenty of space for developing future energy technology along this direction.

关键词： metal hydrogen generation hydrolysis metal water reaction clean energy

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New refrigeration system using CO vapor-solid as refrigerant

HUANG Dongping, DING Guoliang, QUACK Hans

《能源前沿（英文）》 2008年第2卷第4期页码 494-498 doi: 10.1007/s11708-008-0070-x

摘要： A refrigerant must be in the vapor-liquid phase in a vapor-compression refrigeration system, therefore, CO cannot be used as a refrigerant for temperatures lower than -56°C because solid CO will form under the triple point temperature of -56°C. A refrigeration system with CO vapor-solid particles as refrigerant is put forward, by which a temperature lower than the triple point is achieved. An adjustable nozzle, a sublimator, a high-pressure regulating valve and a low-pressure regulating valve are used to replace the conventional evaporator. Theoretical cycle analysis of the refrigeration system shows that its COP can be 50% higher than that of the conventional one.

关键词： refrigerant adjustable temperature vapor-compression refrigeration sublimator

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Human health ambient water quality criteria for 13 heavy metals and health risk assessment in Taihu Lake

《环境科学与工程前沿（英文）》 2022年第16卷第4期 doi: 10.1007/s11783-021-1475-6

摘要：

• The concentrations of 13 heavy metals in Taihu Lake were analyzed.

关键词： Heavy metals Human health ambient water quality criteria Taihu Lake Health risk assessment Contribution rate

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Factors influencing water quality indices in a typical urban river originated with reclaimed water

Jiao Zhang, Zhen Wei, Haifeng Jia, Xia Huang

《环境科学与工程前沿（英文）》 2017年第11卷第4期 doi: 10.1007/s11783-017-0943-5

摘要： The water quality in a typical urban river segment originated with reclaimed water in Beijing was monitored for two years to investigate the evolution of water quality along the river, and statistical analysis was applied to determine factors influencing water quality of such river recharged by reclaimed water. It was found that no significant change in pollutant concentrations (including COD, NH -N, TN and TP) was observed during this time, and their average values were close to those of the original reclaimed water. However, turbidity and algal contents fluctuated temporally in the direction of river flow. Statistical analysis showed that turbidity was strongly positively correlated with algal contents for flow rate<0.1 m·s , whereas it was strongly positively correlated with both algal contents and TOC for flow rate>0.1 m·s . It was observed that diatom was the absolute predominant phyla with as the major species. In terms of algal bloom control, the specific growth rate of algae was strongly correlated to temperature, and was influenced by flow rate as well. Compared with two other rivers originated with reclaimed water and one originated with natural water, the Shannon–Wiener index in the objective river was the lowest, with values between 0.7 and 1.6, indicating a high risk for algal bloom. Statistics showed that Shannon–Wiener index was strongly negatively correlated to nutrient salts and cations.

关键词： Reclaimed water Urban river Turbidity Algae Flow rate

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Long term performance of recycled concrete beams with different water–cement ratio and recycled aggregatereplacement rate

Jingwei YING; Feiming SU; Shuangren CHEN

《结构与土木工程前沿（英文）》 2022年第16卷第3期页码 302-315 doi: 10.1007/s11709-022-0803-7

摘要： The purpose of this study is to reveal the service performance of recycled aggregate concrete (RAC) components for different values of water−cement ratio and replacement rate of recycled coarse aggregate (RCA). Generally, the concrete strength decreases with the increase of the replacement rate of RCA, in order to meet the strength requirements when changing the replacement rate of RCA, it is necessary to change the water−cement ratio at the same time. Therefore, the axial compressive strengths of prism with 25 mix proportions, the short-term mechanical properties and long-term deformation properties of reinforced concrete beams were tested respectively by changing water−cement ratio and RCA replacement rate. The bearing capacity and the strain nephogram of samples under different loads were obtained using the Digital Image Correlation (DIC) method, and a self-made gravity loading experimental device was used for long-term deformation investigation. Results showed that the damage pattern of RAC was the same as that of natural aggregate concrete (NAC), but the brittleness was more pronounced. The brittleness of concrete before failure can be reduced more effectively by adjusting the replacement rate of RCA than by adjusting the water−cement ratio. The water−cement ratio has an evident influence on the axial compressive strength and early creep of concrete, while the replacement rate of RCA has a remarkable effect on the long-term deformation of the concrete beams.

关键词： recycled concrete beam the replacement rate of recycled coarse aggregate water–cement ratio digital image correlation